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Abstract: Injecting CO2 into hydrocarbon reservoirs can enhance the recovery of hydrocarbon resources, and simultaneously, CO2 can be stored in the reservoirs, reducing considerable amount of carbon emissions in the atmosphere. However, injected CO2 tends to go through fractures, high-permeability channels and streaks present in reservoirs, resulting in inefficient hydrocarbon recovery coupled with low CO2 storage performance. Conformance treatments with CO2-resistant crosslinked polymer gels were performed in this study to mitigate the CO2 channeling issue and promote the synergy between enhanced oil recovery (EOR) and subsurface sequestration of CO2. Based on a typical low-permeability CO2-flooding reservoir in China, studies were performed to investigate the EOR and CO2 storage performance with and without conformance treatment. The effect of permeability contrast between the channels and reservoir matrices, treatment size, and plugging strength on the efficiency of oil recovery and CO2 storage was systematically investigated. The results indicated that after conformance treatments, the CO2 channeling problem was mitigated during CO2 flooding and storage. The injected CO2 was more effectively utilized to recover the hydrocarbons, and entered wider spectrum of pore spaces. Consequently, more CO2 was trapped underground. Pronounced factors on the synergy of EOR and CO2 storage were figured out. Compared with the treatment size, the CO2 storage efficiency was more sensitive to the plugging strength of the conformance treatment materials. This observation was important for conformance treatment design in CCUS-EOR projects. According to this study, the materials should reduce the channel permeability to make the channel/matrix permeability ratio below 30. The results demonstrate the importance of conformance treatment in maximizing the performance of CCUS-EOR process to achieve both oil recovery improvement and efficient carbon storage. This study provides guidelines for successful field applications of CO2 transport control in CO2 geo-utilization and storage.